I think that there were a lot of hints that Dean started having strong feelings for Cas WAY before seasons six and seven. In season 4, we already know that Cas is emotionally compromised by Dean, that everyone around him comments on it, from Uriel to Anna to Zachariah. But is Dean feeling the love? Oh, yes. Yes and yes.
When I re-watched 4:10,
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In my head canon, Cas fell in love with Dean first, with Dean only realuzing it much, much later. And that moment when Dean gave Cas back his trenchcoat, well, that just about sealed it for me.
LOVE what you wrote here :)
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