As long as I completely ignore the last chapter (you know, the 19 years later thing) I would say Deathly Hallows. That being said, I must admit, too many good characters died in it =/ like, what. Five in one book. And that's just the deaths I remember. (Moody, Dobby, Tonks, Lupin, Fred....)
That or Half-Blood Prince. I had a tiny fear for the
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